Stop a user accessing the Internet - XP Pro.

you can go to..

gpedit.msc and then to users -> admin -> network

may be settings in there... or you can run a login script to disable the network card and set user policy so thye can't enable it again...
 
Or if they are not computer savvy - just put in a fake proxy server details to Tools>Internet Options>Connection>LAN Settings if it is just for kids...
Edit: This just works for disabling Internet Explorer. If you need to block MSN etc then use Andy's suggestion above.
 
Easiest way is via the router.

Depending on if it's a user's machine and noone else uses it, just deny them access from the router, they will need a static IP address
 
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